Frequency shifts in stimulated Raman scattering

Sideward Stimulated Raman Scattering

The SRS of a short laser pulse is important in the contexts of particle acceleration2 and inertial confinement fusion.3,4 In previous studies of the spatiotemporal evolution of SRS,5–13 the Stokes waves were allowed to pass freely through the pulse boundaries. However, the radial ponderomotive force associated with the pulse can expel plasma from the neighborhood of the pulse axis, in which cas...

Multicolor stimulated Raman scattering microscopy

Stimulated Raman scattering (SRS) microscopy has opened up a wide range of biochemical imaging applications by probing a particular Raman-active molecule vibrational mode in the specimen. However, the original implementation with picosecond pulse excitation can only realize rapid chemical mapping with a single Raman band. Here we present a novel SRS microscopic technique using a grating-based p...

Stimulated Raman Scattering in Semiconductor Nanostructures

Transient stimulated Raman scattering in gas mixtures.

We studied, for the first time to our knowledge, transient stimulated Raman scattering in H(2)- D(2) and H(2)- CH(4) gas mixtures excited with 200-fs and 2-ps, 390-nm pulses. Depending on the composition and partial pressure, of those gases, we observed approximately 40 output lines simultaneously. Under optimum conditions a conversion efficiency of as much as 8% in the combination Raman line a...

Femtosecond time-resolved Raman spectroscopy using stimulated Raman scattering

Femtosecond Raman spectroscopy has been developed to investigate ultrafast photoinduced structural changes of materials. Vibrational modes in the photogenerated transient species are measured by stimulated Raman scattering using a Raman pump pulse with narrow bandwidth and a femtosecond supercontinuum probe pulse. The Raman signal can be measured without slowing the temporal response and broade...